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Third harmonic generation of a nonlinear laser Eigen mode of a self sustained plasma channel

Published online by Cambridge University Press:  01 February 2013

K.K. Magesh Kumar*
Affiliation:
Physics Department, Indian Institute of Technology Delhi, New Delhi, India
V.K. Tripathi
Affiliation:
Physics Department, Indian Institute of Technology Delhi, New Delhi, India
*
Address correspondence and reprint requests to: K.K. Magesh Kumar, Physics Department, Indian Institute of Technology Delhi, New Delhi-110016, India. E-mail: mageshkumar2006@gmail.com
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Abstract

The third harmonic generation of a self organized nonlinear laser Eigen mode of a two-dimensional plasma channel with complete electron evacuation from the inner region is investigated. The nonlinearities arise through the ponderomotive force and relativistic mass variations, while the ions are taken to be immobile. The second harmonic ponderomotive force produces electron density oscillations that beat with the oscillatory velocity due to the laser Eigen mode to create a nonlinear current, driving the third harmonic. As a0 increases up to the threshold value amin, at which complete electron evacuation begins in the inner region, the third harmonic amplitude rises rapidly. Above the threshold, as a0 increases, the width of the inner region where there is no third harmonic current, increases and third harmonic amplitude rises less rapidly. The conversion efficiency is found to be in reasonable agreement with the experimental results.

Type
Research Article
Copyright
Copyright © Cambridge University Press 2013

1. INTRODUCTION

Ultrahigh intensity laser plasma interaction has evolved several novel concept and applications, such as, laser-driven electron accelerators (Tajima & Dawson., 1979; Sprangle et al., Reference Sprangle, Esarey, Ting and Joyce1988; Modena et al., 1995; Ting et al., Reference Ting, Moore, Krushelnick, Manka, Esarey, Sprangle, Hubbard, Burris, Fischer and Baine1997), X-ray lasers (Burnett & Enright, Reference Burnett and Enright1990), fast ignitor inertial confinement fusion (Tabak et al., 1994), ion Coulomb explosion, etc. These applications require long laser propagation distances, in excess of Rayleigh length. Various mechanisms have been demonstrated for the guiding of intense laser pulses in plasmas (Kumarappan et al., Reference Kumarappan, Kim and Milchberg2005; Geddes et al., Reference Geddes, Toth, Tilborg, Esarey, Schroeder, Cary and Lee-Mans2005; Malka et al., Reference Malka, Faure, Marques, Amiranoff, Courtois, Najmudin, Krushenick, Salvati, Modena, Najmudin, Dangor, Clayton, Marsh, Joshi, Malka, Darrow, Danson, Neely and Walsh1995; Nikitin et al., Reference Nikitin, Antonsen, Clark, Li and Milchberg1997; Sprangle et al., Reference Sprangle, Esarey, Krall and Joyce1992; Verma & Sharma, Reference Verma and Sharma2009a; Reference Verma and Sharma2009b; Singh & Singh, Reference Singh and Singh2011). A Laser of intensity 5 × 1015 W/cm2 has been channeled up to 3 cm in a preformed plasma waveguide structure created by the hydrodynamic expansion (Durfee & Milchberg, Reference Durfee Iii and Milchberg1993). Jackel et al. (Reference Jackel, Burris, Grun, Ting, Manka, Evans and Kosakowskii1995) guided laser pulse of intensity 1016 W/cm2 using glass capillary waveguides in vacuum and Ehrlich et al. (Reference Ehrlich, Cohen, Zigler, Krall, Sprangle and Esarey1996) used long cylindrical plasma channel formed by a slow capillary discharge. More detailed analyses of self-focusing and channeling of a short relativistic laser pulse has been done by various groups (Sprangle et al., Reference Sprangle, Esarey, Krall and Joyce1992; Bulanov et al., Reference Bulanov, Pegoraro and Pukhov1995; Mora & Antonsen, Reference Mora and Antonsen1996; Sarkisov et al., Reference Sarkisov, Bychenkov, Novikov, Tikhonchuk, Maksimchuk, Chen, Wagner, Mourou and Umstadter1996; Borisov et al., Reference Borisov, Borovskiy, Shiryaev, Korobkin, Prokhorov, Solem, Luk, Boyer and Rhodes1992).

Sun et al. (Reference Sun, Edward, Lee and Guzdar1987) and Borisov et al. (Reference Borisov, Borovskiy, Shiryaev, Korobkin, Prokhorov, Solem, Luk, Boyer and Rhodes1992) have studied the nonlinear propagation of intense ultrashort cylindrically symmetric laser beam in cold underdense plasma, allowing for complete electron evacuation on the axis. Macchi et al. (Reference Macchi, Bigongiari, Ceccherini, Cornolti, Liseikina, Borghesi, Kar and Romagnani2007) studied the propagation of an intense laser pulse in an underdense, inhomogeneous plasma on the time scale of several picoseconds. They addressed the effects of the ion dynamics following the charge-displacement self-channeling of the laser pulse. Pathak and Tripathi (Reference Pathak and Tripathi2006) have studied nonlinear eigen mode of a plasma channel and examined its stability to stimulated Raman Scattering. However, the treatment is limited to intensities where electron hole is not created on the axis.

In this paper, we examine the issue of harmonic excitation of a self guided nonlinear laser eigen mode in a plasma, where complete electron evacuation occurs on the axis. Needless to mention, harmonic generation is one of the most dominating nonlinear effects induced by linearly polarized intense short pulse laser in a plasma. Third harmonic is particularly important as observed in several experiments (Lin et al., Reference Lin, Chen, Pai, Kuo, Lee, Wang, Chen and Lin2006; Kuo et al., Reference Kuo, Pai, Lin, Lee, Lin, Wang and Chen2007; Sunstov et al., Reference Suntsov, Abdollahpour, Papazoglou and Tzortzakis2010; Ganeev et al., Reference Ganeev, Boltaev, Tugushev, Usmanov, Baba and Kuroda2010; Yang et al., Reference Yang, Zhang, Zhang, Zhao, Li, Teng, Li, Wang, Chen, Wei, Ma, Yu and Sheng2003). Liu et al. (Reference Liu, Umstadter, Esarey and Ting1993) have used the pump-probe technique to observe third harmonic generation in a preformed plasma. Nitikant and Sharma (Reference Nitikan and Sharma2004) examined the resonant second-harmonic generation of a Gaussian laser short pulse undergoing periodic self-focusing in a preformed plasma. Ganeev et al. (Reference Ganeev, Boltaev, Tugushev, Usmanov, Baba and Kuroda2010) experimentally observed the third harmonic generation of picosecond and femtosecond laser pulses in plasma plumes. They showed that the technique can be used for generation of harmonics in the shorter wavelength range. Yang et al. (Reference Yang, Zhang, Zhang, Zhao, Li, Teng, Li, Wang, Chen, Wei, Ma, Yu and Sheng2003) have obtained an efficiency conversion greater than 0.1 percent of a strong third-harmonic emission from a plasma channel that is formed by self-guided propagation of femtosecond laser pulses in air. Similarly, Sunstov et al. (Reference Suntsov, Abdollahpour, Papazoglou and Tzortzakis2010) studied the third-harmonic generation in air by a filamented femtosecond infrared laser pulse propagating through a thin plasma channel. Verma and Sharma (Reference Verma and Sharma2009a; Reference Verma and Sharma2009b) have studied third harmonic generation by a finite spot size laser in a tunnel ionizing gas with density rising in a stepwise manner. Gupta et al. (Reference Gupta, Sharma and Mahmoud2007) have investigated the generation of plasma wave and third harmonic generation at ultra relativistic laser power and obtained power of the third harmonic generation. Garg and Tripathi (Reference Garg and Tripathi2010) have studied resonant third harmonic generation in a semiconductor slab with density ripple of wave number q. Verma and Sharma (Reference Verma and Sharma2011) obtained the mode structure of right circularly polarized nonlinear laser Eigen mode in a self created plasma channel in the presence of an axial magnetic field and Ghorbanalilu (Reference Ghorbanalilu2012) studied second and third harmonics generation in a strongly magnetized dense plasma.

Here we develop a two-dimensional slab model for nonlinear eigen mode of a ponderomotive force driven plasma channel, with perfect electron hole on the axis and study third harmonic generation of the eigen mode. The relativistic mass increase is self consistently incorporated while ions are taken to be immobile. In the axial region, the laser ponderomotive force exceeds ion space charge force on electrons, hence complete electron evacuation up to a width is obtained. Beyond this width, the ponderomotive force is balanced by space charge force. The relativistic mass nonlinearity adds to non-uniformity of the channel. The second harmonic component of ponderomotive force induces longitudinal oscillatory velocity on electrons and gives rise to second harmonic electron density perturbation. The latter couples with oscillatory velocity due to the laser to produce a nonlinear third harmonic current giving third harmonic radiation.

In Section 2, we study the mode structure of two-dimensional laser eigen mode in the self created plasma channel. In Section 3, we study the third harmonic generation of the self consistent laser eigen mode and estimate its efficiency. The results are discussed in Section 4.

2. NONLINEAR LASER EIGEN MODE

Consider a singly ionized cold collionless plasma of uniform electron density n 00. A two-dimensional intense short pulse laser propagates through it along $\hat{z}$ with fast phase variation as,

(1)$${\bf E}=\hat{y} A_T\lpar x\rpar e^{-i\lpar {\rm \omega} t-k_z z\rpar }.$$

The duration of the pulse is larger than the electron plasma period but much shorter than the ion plasma period, so that the ions remain immobile. We look for a suitable profile of A T (x) that would propagate without convergence or divergence and allow A T to acquire relativistically large values. The laser imparts oscillatory velocity to electrons, $\vec v=$$e{\bf E}/mi{\rm \omega} {\rm \gamma}$, where ${\rm \gamma}=\sqrt{1+a^2/2}\comma \; a=e \vert A_T \vert /m{\rm \omega} c\comma \; -e$ and m are the electronic charge and rest mass, and c is the speed of light in vacuum. The laser exerts a ponderomotive force on electrons,

(2)$${\bf F}_{\bf p}=e \nabla {\rm \phi}_p\comma \;$$

where ${\rm \phi}_p=-({mc^2 / e}) \lpar \sqrt {1+a^2/2}-1 \rpar.$ For an eigen mode, field amplitude does not change with z, hence the ponderomotive force has only x− component. It pushes the electrons outward (to higher values of |x|) producing a space charge field Es = −∇ϕs. The radial movement of electrons takes place as long as $\vec F_p \gt e \vec E_s$. On the time scale of a plasma period ω−1p, a quasi-steady state is reached when Fp = e Es, or ϕs = −ϕp. From the Poisson's equation,

(3)$$\nabla^2 {\rm \phi}_s=4{\rm \pi} e\lpar n_e-n_0^0\rpar \comma \;$$

one may write, using ϕs = −ϕp, the modified electron density

(4)$$n_e=n^0_0 - {1\over 4{\rm \pi} e} \nabla^2 {\rm \phi}_p\comma \;$$

where n 00 is the ion density (equal to unperturbed electron density). Since, n e cannot be negative, Eq. (4) is valid only as long as

(5)$$n^0_0 \gt {1\over 4{\rm \pi} e}\nabla^2 {\rm \phi}_p.$$

Thus, the electron density in the channel can be written as,

(6)$$n_e = \left\{\matrix{0 & \hbox{for} x \lt r_{0p} \cr n_0^0 - {1 \over 4{\rm \pi} e}\nabla ^2 {\rm \phi} _p & {\rm for} x \gt r_{0p}}\right. \comma \;$$

where r 0p is the value of x at which

(7)$${\partial^2 \over \partial x^2} \left. \sqrt{1+{\vert E_y \vert^2e^2 \over 2m^2{\rm \omega}^2c^2}}\right\vert_{x\,=\,r_{0p}} = -{\rm \omega}^2_p/c^2\comma \;$$

where ${\rm \omega}_p=\sqrt{4{\rm \pi} n^0_0 e^2/m}=k_{\,p}c.$ One may note that the electron density increases from zero at |x| = r 0p to higher values as |x| increases.

For x < r 0p (for a symmetric mode), the laser field E y may be written as,

(8)$$E_y=A_0 cos\lpar {\rm \alpha} x\rpar e^{-i\lpar {\rm \omega} t-k_{z}z\rpar }\comma \;$$

where A 0 is the amplitude of the laser at x = 0 and ${\rm \alpha}=\sqrt{({{\rm \omega}^2 / c^2})-k^2_z}.$ For x > r 0p, E y is governed by the wave equation

(9)$${\partial^2 \over \partial x^2}E_y+ \left[{{\rm \omega}^2\over c^2}\left(1-{{\rm \omega}^2_p \over {\rm \omega}^2}{n_e\over {\rm \gamma} n^0_0}\right)-k^2_z \right]E_y=0.$$

The term ${\rm \omega}^2_p({ne/ {\rm \gamma} n^0_0})$ in the wave equation arises due to the contribution of current density, $\vec J = -n_e e \vec v$ driven by the laser pulse and $\vec v\lpar \!= \hat{y} e E_y/mi{\rm \omega} {\rm \gamma}\rpar $ is the oscillatory velocity imparted by the laser.

Using E y from Eq. (1) in Eq. (9), writing A T = A e iϕ with A and ϕ real, and separating out the real and imaginary parts of Eq. (9), we obtain

$$\displaystyle{d \over dx} \left(A^2 \displaystyle{d {\rm \phi} \over dx} \right)= 0 \Rightarrow A^2 \displaystyle{d {\rm \phi} \over dx} = constant = C_1\comma \;$$
(10)$$\displaystyle{d^2 A \over dx^2} - \displaystyle{C_1^2 \over A^3} + \left[\displaystyle{{\rm \omega}^2 \over c^2} \left(1 - \displaystyle{{\rm \omega}_p^2 \over {\rm \omega}^2} \displaystyle{n_e \over {\rm \gamma} n_0^0}\right)- k_z^2\right]A = 0.$$

One may multiply Eq. (10) by e/mωc and write it for normalized amplitude a = eA/mωc as,

(11)$$\displaystyle{d^2 a \over dx^2} - \displaystyle{C_1^2 \over a^3} + \left[\displaystyle{{\rm \omega}^2 \over c^2} \left(1 - \displaystyle{{\rm \omega}_p^2 \over {\rm \omega}^2} \displaystyle{n_e \over {\rm \gamma} n_0}\right)- k_z^2\right]a = 0.$$

Using the value of n e/n 00 from Eq. (4),

(12)$$\displaystyle{n_e \over n_0^0} = 1 + \displaystyle{c^2 \over 2{\rm \omega}_p^2} \left(\displaystyle{a \over \sqrt{1 + a^2/2}} \displaystyle{d^2 a \over dx^2} + \displaystyle{1 \over \lpar 1 + a^2/2\rpar ^{3/2}}\left(\displaystyle{da \over dx}\right)^2\right)\comma \;$$

Eq. (11) can be written as

(13)$$\eqalign{& \displaystyle{d^2 a \over dx^2} - {C_1^2 \over a^3} \lpar 1 + a^2/2\rpar - \displaystyle{a \over 2\lpar 1 + a^2/2\rpar } \left(\displaystyle{da \over dx}\right)^2 \cr & + \left[\displaystyle{{\rm \omega}^2 \over c^2}\left(1 - \displaystyle{{\rm \omega}_p^2 \over {\rm \omega}^2 \sqrt{1 + a^2/2}}\right)- \displaystyle{k_z^2 c^2 \over {\rm \omega}^2}\right]\lpar 1 + a^2/2\rpar a = 0.}$$

As x → ∞, the nonlinear terms vanish and a → 0. The equation will remain well behaved only when C1 = 0. At x = r 0p, n e/n 00 = 0, Eq. (12) gives

(14)$$\displaystyle{d^2 a \over dx^2} = - \displaystyle{2 \sqrt{1 + a^2/2} \over a} \left[\displaystyle{{\rm \omega}_p^2 \over c^2} + \displaystyle{1 \over 2\lpar 1 + a^2/2\rpar ^{3/2}} \left(\displaystyle{da \over dx}\right)^2\right]\comma \;$$

while from Eq. (11), on putting ne/n00 = 0, and C 1 = 0, we get

(15)$$\displaystyle{d^2 a \over dx^2} = \left(\displaystyle{{\rm \omega}^2 \over c^2} - k_z^2\right)a.$$

Comparing Eq. (14) and (15), we obtain,

(16)$$\displaystyle{1 \over 2\lpar 1 + a^2/2\rpar ^{3/2}} \left(\displaystyle{da \over dx}\right)^2 = \left(\displaystyle{{\rm \omega}^2 \over c^2} - k_z^2 \right)\displaystyle{a^2 \over 2 \sqrt{1 + a^2/2}} - \displaystyle{{\rm \omega}_p^2 \over c^2}.$$

We want a and da/dx to be continuous at x = r 0p, hence

(17)$$\eqalign{& \quad \quad a = a_0 cos\lpar {\rm \alpha} {r_{0p}}\rpar \comma \; \cr & \displaystyle{da \over dx} = - a_0 {\rm \alpha} sin\lpar {\rm \alpha} {r_{0p}}\rpar .}$$

Using these in Eq. (16) we get an equation governing r 0p,

(18)$$\displaystyle{a_0^2 {\rm \alpha}^2 sin^2 \lpar {\rm \alpha} {r_{0p}}\rpar \over 2\lpar 1 + \lpar a_0^2/2\rpar \lpar cos {\rm \alpha} {r_{0p}}\rpar ^2\rpar ^{3/2}} = \displaystyle{\lpar {\rm \omega}^2/c^2 - k_z^2\rpar a_0^2 cos^2 {\rm \alpha} {r_{0p}} \over 2 \sqrt{1 + \lpar a_0^2/2\rpar \lpar cos^2 {\rm \alpha} {r_{0p}}\rpar }} - \displaystyle{{\rm \omega}_p^2 \over c^2}\comma \;$$

One must choose k z < ω/c, ωp to be small and a 0 such that the right hand side is +ve. Eq. (18) can be written as,

(19)$$\displaystyle{{\rm \alpha}^2 c^2 \over {\rm \omega}^2} = \displaystyle{2 {\rm \omega}_p ^2 \over {\rm \omega}^2} \displaystyle{\sqrt{1 + \lpar a_0^2/2\rpar cos^2 \lpar {\rm \alpha} {r_{0p}}\rpar } \over a_0^2 cos^2 \lpar {\rm \alpha} {r_{0p}}\rpar } + \displaystyle{\lpar {\rm \alpha}^2 c^2 / {\rm \omega}^2\rpar tan^2 \lpar {\rm \alpha} {r_{0p}}\rpar \over 1 + \lpar a_0^2/2\rpar \lpar cos^2 \lpar {\rm \alpha} {r_{0p}}\rpar }.$$

To obtain r 0p and α explicitly for a given ωp/ω, we proceed as follows. At some large value of x we chose a small value of a. Now pick a value of ck z/ω and take da/dx = −α′a, where ${\rm \alpha}^\prime=\lpar k^2_z+({{\rm \omega}^2_p / c^2})- ({{\rm \omega}^2 / c^2})\rpar ^{1/2}.$ Solve Eq. (13) backward to smaller x, up to a point where n e = 0, i.e., Eq. (16) is satisfied. Call this point x = r 0p. At this point, the continuity conditions (17) demand, (1/a)(da/dx) = −αtanr 0p). If this condition is not met, we try a different value of ck z/ω and repeat the same procedure until this condition is satisfied. Once we get a suitable ck z/ω and have r 0p, α, Eq. (19) gives the value of a 0.

We have plotted the hole half width of the electron (equivalent to hole radius) r 0pωp/c with a 0 in Figure 1 and ck z/ω with a 0 in Figure 2. The hole radius increases rapidly with a 0 in the range of a 0 → 1–4 with a strong dependence on ωp/ω and tends to saturate for larger values of a 0. With increase in ωp/ω, the electron density on the shoulders of the channel increases resulting in considerable reduction in channel radius. From Figure 1 one may note that beyond a certain value of a 0(= a min) the electrons are completely removed from the axis forming an electron hole. The value a min increases with increase in ω/ωp and electron evacuation does not occur for a min < 1. With increase in laser amplitude, as the hole size increases, there is corresponding reduction in the phase velocity of the eigen mode (see Fig. 2). This is because the effective refractive index increases with increase in laser amplitude a 0. The dispersion relation is plotted in Figure 3 for a 0 = 2(dot), 3(solid). One may note that the eigen frequency shows a monotonous increase with wave vector of the mode with a strong dependence on a 0. For ω/ωp = 1.2, k zcp = 0.525 and a 0 = 2, the phase velocity of the eigen mode turns out to be ω/k zc = 2.25 and the value of ω/k zc decreases with a 0 as mentioned earlier. Figure 4 shows the mode structure, |a/a 0|2 versus normalized distance k px, for a 0 = 3, ω/ωp = 1.2, k zcp = 0.9 and k pr 0p = 1. The eigen mode field varies cosinudally inside the channel (shown by solid line) and starts decaying from channel boundary (shown by dashed line) at k px = k pr 0p = 1. The mode intensity |a/a 0|2 falls off to half of its axial value at k pr 0p = 1. The intensity decreases more rapidly inside the electron hole and near the channel boundary. Outside the channel, it decreases slowly. The value of |a|2 reduces to 1/10 of its axial value at k px = 1.5.

Fig. 1. Variation of normalized channel radius r 0pωp/c with laser amplitude a 0 for ωp/ω = 0.86 (dot) and 0.83 (solid).

Fig. 2. Variation of k zc/ω (inverse of phase velocity of eigen mode) with a 0 for ω/ωp= 1.2.

Fig. 3. Variation of ω/ωp with k zcp for a 0 = 2 (dot) and 3 (dash).

Fig. 4. Variation of |a/a 0|2 with k px for a 0 = 2, ω/ωp = 1.2, k zcp = 0.9, and k pr 0p = 1.

The power contained in the eigen mode per unit y width is,

(20)$$P = \displaystyle{m^2 c^4 {\rm \omega}^2 {\rm \epsilon}_0 \over 2e^2} \int_0^{\infty} \vert a\vert ^2 dx.$$

where |a|2 is the laser eigen mode intensity obtained by solving Eq. (13) as mentioned earlier. Multiplying both sides of Eq. (20) by cp, one obtains the normalized power,

(21)$$\displaystyle{Pc/{\rm \omega}_p \over P_0} \,=\,\, \int_0^{\infty} \vert a\vert ^2 dx = \int_0^{r_{0p}} \vert a\vert ^2 dx + \int_{r_{0p}}^{\infty} \vert a\vert ^2 dx.$$

where $P_0=({{\rm \omega}^2/ {\rm \omega}^2_p})({m^2 c^5 \epsilon_0\! / 2e^2})=3.47{\left({\rm \omega} / {\rm \omega}_p\right)}^2\times10^9 W$ and x → xωp/c. Figure 5 shows the variation of normalized power $(Pc/{\rm \omega}_p)/ P_0$ with a 0. The normalized power $(Pc/{\rm \omega}_p)/ P_0$ varies almost linearly with a 0. For a 0 = 1.5, ωp/ω = 0.83, the power turns out to be $Pc/{\rm \omega}_p=$$1.6{\left({\rm \omega} / {\rm \omega}_p\right)}^2 \times 10^{10}W.$ Hence for a 0 = 1.5, the power obtained is slightly less than the critical power $\lpar P_c=1.78{\left({\rm \omega} / {\rm \omega}_p\right)}^2 \times 10^{10}W)$ needed for the formation of electron hole. Thus for the electrons to be completely removed from the axis, a 0 must be kept higher for the same value of ωp/ω such that the condition P/P cr ≥ 1 is achieved. Increasing the value of a 0 from 2 to 5 the normalized power $(Pc/{\rm \omega}_p )/ P_0$ increases by a factor of 2. How ever with increase in ωp/ω, $(Pc/{\rm \omega}_p)/ P_0$ decreases, so as r 0p. For a 0 = 5, ωp/ω = 0.83 and r 0p = 1.38cp, the normalized power $(Pc/{\rm \omega}_p )/ P_0$ turns out to be 9.0058, which is very close to the value obtained by Sun et al. Reference Sun, Edward, Lee and Guzdar1987. Hence, the power contained in the eigen mode for a 0 = 5 is $Pc/{\rm \omega}_p=$$3.948{\left({\rm \omega}/{\rm \omega}_p\right)}^2 \times 10^{10}W$, exceeding the critical power P cr by a factor of 2.

Fig. 5. Variation of the normalized power $(Pc/{\rm \omega} p)/ P_0$ with a 0 for ω/ωp = 1.2 and k zcp = 0.9.

3. THIRD HARMONIC GENERATION

The laser eigen mode (E y) propagating through the plasma channel with density profile given by Eq. (6) exerts a second harmonic ponderomotive force on electrons,

(22)$${\bf F}_{2{\rm \omega}} = -\lpar 1/2\rpar e\!\mathop {{\rm v}} \limits^{\rightarrow} \times {\bf B} = - {\hat z} \displaystyle{e^2 k_z E_y^2 \over 2 mi{\rm \omega}^2 {\rm \gamma}}.$$

Using this in the equations of motion and continuity one obtains the oscillatory velocity $\vec{v}_{2{\rm \omega}}$ and density n .

(23)$$\vec{v}_{2{\rm \omega}} = - \displaystyle{{\bf F}_{2 {\rm \omega}} \over mi2{\rm \omega} {\rm \gamma}} = - {\hat z} \displaystyle{e^2 k_z E_y^2 \over 4 m^2 {\rm \omega}^3 {\rm \gamma}^2}\comma \;$$
(24)$$n_{2{\rm \omega}} =\displaystyle{n_e k_z {\rm v}_z \over {\rm \omega}} = - \displaystyle{n_e e^2 k_z^2 E_y^2 \over 4 m^2 {\rm \omega}^4 {\rm \gamma}^2}.$$

The density perturbation n couples with oscillatory velocity $\vec{v}$ to produce nonlinear current density at the third harmonic frequency (3ω),

(25)$${\bf J}^{NL} = - \lpar 1/2\rpar n_{2{\rm \omega}} e\!\mathop{{\rm v}}\limits^{\rightarrow} = - {\hat y} \displaystyle{{\rm \omega}_p^2\lpar n_e/n_0^0\rpar k_z^2 c^2 \over 8i {\rm \omega}^{4} {\rm \gamma}^2} a^2 {\rm \omega} {\rm \epsilon}_0 E_y\comma \;$$

where a = e|E y|/mωc. The nonlinear third harmonic current density produces third harmonic electric field E. This field produces self consistent current density J L,

(26)$${\bf J}_{3{\rm \omega}}^L = i \displaystyle{n_0^0 e^2 {\bf E}_{3{\rm \omega}} \over 3 m{\rm \omega} {\rm \gamma}}.$$

The wave equation governing E can be deduced from Maxwell's equations,

(27)$$\nabla \times {\bf E}_{3{\rm \omega}} = 3i{\rm \omega}{\bf B}_{3{\rm \omega}}\comma \;$$
(28)$$\nabla \times {\bf B}_{3{\rm \omega}} = - 3i{\rm \omega} {\rm \mu}_0\lpar {\bf J}^{NL} + {\bf J}_{3{\rm \omega}}^{L}\rpar - i \displaystyle{3{\rm \omega} \over c^2} {\bf E}_{3{\rm \omega}}.$$

Since J NL is parallel to $\hat{y}$ (cf. Eq. (25)), E is also parallel to $\hat{y}$. Defining a  = e E 3ωy/mωc and taking fast t,z variation as e zi(3ωtk 3zz), we obtain from Eqs. (25)–(28),

(29)$$\eqalign{& \displaystyle{d^2 a_{3{\rm \omega}}\over dx^2} + 2ik_{3z} \displaystyle{\partial a_{3{\rm \omega}} \over \partial z} + \left(\displaystyle{9 {\rm \omega}^2 \over c^2} - \displaystyle{{\rm \omega}_p^2 \lpar n_e/n_0^0\rpar \over c^2 {\rm \gamma}} - k_{3z}^2\right) \times \cr & \quad a_{3{\rm \omega}} = \displaystyle{3 \over 8} a^3\lpar k_z c/{\rm \omega}\rpar ^2 \displaystyle{{\rm \omega}_p^2 \lpar n_e/n_0^0\rpar \over {\rm \gamma}^2 c^2}.}$$

One may note that the nonlinear third harmonic source current density is finite only in the outer region |x| > r 0p. It excites a number of eigen modes in the channel at the third harmonic. We consider the excitation of the fundamental mode of the third harmonic that has the mode structure similar to that of the pump laser,

(30)$$a_{3{\rm \omega}} = eE_{3{\rm \omega} y}/m{\rm \omega} c = A_{3{\rm \omega}}\lpar z\rpar F\lpar x\rpar e^{-i\lpar 3{\rm \omega} t-k_{3z}z\rpar }\comma \;$$
(31)$$F \lpar x \rpar = \left\{\matrix{a_0 cos \lpar {\rm \alpha} x \rpar & \hbox{for} \, 0 \lt \vert x \vert \lt {r_{0p}} \cr a \lpar x \rpar & \hbox{for} \, \vert x \vert \gt {r_{0p}}}. \right.$$

where $k_{3z}=\sqrt{{9{\rm \omega}^2 \over c^2}-{\rm \alpha}^2}.$

Substituting Eq. (30) in (29), multiplying the resulting equation by F(x) *dx and integrating from −∞ to ∞, we obtain,

(32)$$\displaystyle{\partial A_{3{\rm \omega}}\over \partial z} - i {\rm \beta} A_{3{\rm \omega}} = \displaystyle{3 \over 16ik_{3z}} \left(\displaystyle{k_z c \over {\rm \omega}}\right)^2 \displaystyle{{\rm \omega}_p^2 \over c^2}Ge^{-i\lpar 3k_z - k_{3z}\rpar z}\comma \;$$

where ${\rm \beta}={1 \over 2k_{3z}}\left[{8 {\rm \omega}^2 \over c^2}+{k^{2}_{z}}-{k^{2}_{3z}}\right]\comma \; G={\int^{\infty}_{- \infty} a^3\lpar x\rpar \lpar \lpar ne/n^0_0\rpar /{\rm \gamma}^2\rpar F\lpar x\rpar ^{\ast} {dx} \over \int^{\infty}_{-\infty}\vert F\lpar x\rpar \vert^{2} dx}.$

Effectively the integral in the numerator of G is the sum of two integrals one with limits −∞ to −r 0p and then from r 0p to ∞ as there are no electrons (n e = 0) in the inner region. One may solve Eq. (32) on taking ∂/∂z = −iδ, δ = (3k z − k 3z). Hence,

(33)$$\eqalign{& A_{3{\rm \omega}}\lpar z\rpar \cr & = \displaystyle{3\lpar k_z c/{\rm \omega}\rpar ^2 Ge^{-i\lpar {\rm \beta}+3k_z - {k_{3z}}\rpar z} \over 16[ 8\lpar {\rm \omega}/{\rm \omega}_p\rpar ^2 + \lpar k_z c/{\rm \omega}_p\rpar ^2 - 3\lpar {k_{3z}}c/{\rm \omega}_p\rpar ^2 + \lpar 6k_{3z} c/{\rm \omega}_p\rpar \lpar k_z c/{\rm \omega}_p\rpar ] }\comma \; }$$
(34)$$ \left \vert \displaystyle{a_{3{\rm \omega}} \over a_0}\right\vert^2 = \left(\displaystyle{3\lpar k_z c/{\rm \omega}\rpar ^2 G \over \matrix{16 [ 8 \lpar {\rm \omega}/{\rm \omega}_p \rpar ^2 + \lpar k_z c/{\rm \omega}_p \rpar ^2 \cr \quad- 3 \lpar {k_{3z}}c/{\rm \omega}_p\rpar ^2 + \lpar 6k_{3z} c/ {\rm \omega}_p \rpar \lpar k_z c/{\rm \omega}_p\rpar ] }}\right)^2.$$

In the fundamental mode, the amplitude of the third harmonic is maximum at the channel axis. The efficiency of the third harmonic shows a strong relationship with laser amplitude a 0 and frequency ω. Figure 6 shows the variation of axial amplitude of the third harmonic with normalized laser frequency ω/ωp for a 0 = 3. With increase in normalized laser frequency ω/ωp the fundamental and third harmonic wave vectors k zcp, k 3zcp(≈ 3ω/ωp) and inverse of the phase velocity k zc/ω increases. Hence the denominator in Eq. (34) decreases steadily, whereas the numerator monotonously increases with ω/ωp. The third harmonic efficiency |a 3 ω/a 0|2 at constant a 0 shows a gradual increase in the range of ω/ω → 1.1–1.3 and increases bit faster beyond ω/ωp = 1.3. Beyond ω/ωp = 1.3 the denominator in Eq. (34) attains a fairly constant value.

Fig. 6. Variation of the square of normalized third harmonic amplitude | a /a 0|2 with ω/ωp for a 0 = 3.

From Figure 7 one may note that the efficiency gradually increases with the laser amplitude a 0 for ω/ωp = 1.2. However with the increase in a 0, the cavitation radius r 0p increases and increasing r 0p adversely effects the growth of third harmonic efficiency |a /a 0|2. But the laser intensity amplitude a 20 is predominant both inside and outside the channel. Hence with increase in the laser amplitude a 0 the lowering of third harmonic efficiency due to increasing r 0p can be compensated. However beyond a 0 = 3, the channel radius r 0p tends to saturate and the third harmonic efficiency grows with a 0.

Fig. 7. Variation of the square of normalized third harmonic amplitude | a /a 0|2 with a 0 for ω/ωp = 1.2 and k zcp = 0.9.

To validate the efficacy of our analytical calculation we compare our results with the experimental results obtained by Kuo et al. (Reference Kuo, Pai, Lin, Lee, Lin, Wang and Chen2007). Kuo et al. (Reference Kuo, Pai, Lin, Lee, Lin, Wang and Chen2007) have experimentally demonstrated the enhancement of relativistic third-harmonic generation in both uniform and rippled density plasma waveguide using linearly polarized laser beam of amplitude a 0 = 1. For the axially uniform channel case, they have obtained an efficiency of 1.1 × 10−8 at plasma density n 00 = 4.8 × 1018 cm −3. For a comparison, we may calculate the conversion efficiency from Eq. (31) for the parameters: ωp/ω0.05 (corresponding to n 00 = 4.8 × 1018 cm −3 at 1μm laser wavelength) and a 0 = 1.5. The conversion efficiency |a /a 0|2 of third harmonic for the aforementioned parameters turns out to be 1.95 × 10−8, which are within a factor of 2 from Kuo et al. (Reference Kuo, Pai, Lin, Lee, Lin, Wang and Chen2007). However the efficiency of the third harmonic can be improved by increasing the laser frequency or by increasing the laser amplitude a 0 as shown in Figures 6 and 7.

4. CONCLUSIONS

A self consistent non-paraxial formalism of laser guiding in a self created channel with a perfect hole in the interior, developed here reveals that inside the hole, in two dimensions, the laser field is sinusoidal in x while its amplitude falls off with x beyond x = r 0p. The radius of the hole r 0p increases with normalized laser amplitude and tends to saturate for large values of a 0. The frequency of the eigenmode ω increases with wave vector k z with a strong dependence on laser amplitude a 0. The power contained in the laser eigen mode is found to vary almost linearly with a 0

The laser eigen mode produces linearly polarized third harmonic outside and inside the electron cavity. The conversion efficiency of the laser eigen mode into the fundamental radial eigen mode of the third harmonic |a 3 ω/a 0|2 shows a gradual increases as ω/ωp increases from 1.1 to 1.3 and sharply increases beyond ω/ωp = 1.3. The third harmonic conversion efficiency increases with a 0 more than linearly. For the parameters of the experiment by (Kuo et al., Reference Kuo, Pai, Lin, Lee, Lin, Wang and Chen2007) the conversion efficiency in a unrippled plasma calculated by our model is in reasonable agreement with the experimental result.

ACKNOWLEDGEMENT

One of the authors, Magesh would like to thank IIT Delhi for financial support.

References

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Figure 0

Fig. 1. Variation of normalized channel radius r0pωp/c with laser amplitude a0 for ωp/ω = 0.86 (dot) and 0.83 (solid).

Figure 1

Fig. 2. Variation of kzc/ω (inverse of phase velocity of eigen mode) with a0 for ω/ωp= 1.2.

Figure 2

Fig. 3. Variation of ω/ωp with kzcp for a0 = 2 (dot) and 3 (dash).

Figure 3

Fig. 4. Variation of |a/a0|2 with kpx for a0 = 2, ω/ωp = 1.2, kzcp = 0.9, and kpr0p = 1.

Figure 4

Fig. 5. Variation of the normalized power $(Pc/{\rm \omega} p)/ P_0$ with a0 for ω/ωp = 1.2 and kzcp = 0.9.

Figure 5

Fig. 6. Variation of the square of normalized third harmonic amplitude | a/a0|2 with ω/ωp for a0 = 3.

Figure 6

Fig. 7. Variation of the square of normalized third harmonic amplitude | a/a0|2 with a0 for ω/ωp = 1.2 and kzcp = 0.9.