1. INTRODUCTION
The problem of intense short-pulse laser–plasma interaction has been an active area of research. Among them, non-linear phenomenon of harmonic generation has been interested by many researchers from 1961 up to now (Franken et al., Reference Franken, Hill, Peters and Weinreich1961; Grebogi et al., Reference Grebogi, Tripathi and Chen1983; Esarey et al., Reference Esarey, Ting, Sprangle, Umstadter and Liu1993; Ondarza-Rovira & Boyd, Reference Ondarza-Rovira and Boyd2000; Földes et al., Reference Földes, Kocsis, Rácz, Szatmári and Veres2003; Racz et al., Reference Racz, Foldes, Kocsis, Veres, Eidmann and Szatmri2006; Cairns, Reference Cairns2009). In process of high-order harmonic generation, second harmonics (SH) has a unique place because of many applications such as extreme ultraviolet non-linear optics (Yeung et al., Reference Yeung, Rykovanov, Bierbach, Li, Eckner, Kuschel, Woldegeorgis, Rödel, Sävert, Paulus, Coughlan, Dromey and Zepf2017), laser–plasma interaction properties, X-ray sources (Giulietti et al., Reference Giulietti, Banfi, Deha, Giulietti, Lucchesi, Nocera and Zun2009), etc. On the other hand, the generation of magnetic fields during high-intensity laser–plasma interaction is a subject that has been under investigation for many years (Lehner, Reference Lehner1994; Berezhiani et al., Reference Berezhiani, Mahajan and Shatashvili1997; Gorbunov et al., Reference Gorbunov, Mora and Antonsen1997; Zheng et al., Reference Zheng, Zhu and He2000; Kato et al., Reference Kato, Nakamura, Mima, Sentoku, Nagatomo and Owadano2004). This subject has motivated an ingoing strong effort to analysis of laser interaction with magnetized plasmas.
A magnetic field with proper configuration may be employed for efficient SH generation by providing the additional momentum, which is essential for phase matching (Kant & Sharma, Reference Kant and Sharma2004; Askari & Noroozi, Reference Askari and Noroozi2009, Reference Askari and Azish2011; Vaziri (Khamedi) et al., Reference Vaziri (Khamedi), Sohailya and Bahrampour2015). When a magnetic field is applied into a plasma, the electron dynamic is modified, and this leads to the non-linear current modification. Therefore, it is reasonable that the magnetic field affects the harmonics generation. The magnetic field could have additive (Kant & Thakur, Reference Kant and Thakur2016) or destructive (Sharma & Sharma, Reference Sharma and Sharma2012; Kuri & Das, Reference Kuri and Das2016) role on SH conversion efficiency in interaction of laser-magnetized plasma. When the density perturbation produced by magnetic field is coupled with electron quiver motions, it is plausible to generate the SH (Jha et al., Reference Jha, Mishra, Raj and Upadhyay2007). It has been shown that the SH power is increased by increasing the magnetic field strength in normal radiation of a linearly polarized laser pulse with a magnetized plasma; however, the magnetic field was essential for SH generation. On the other hand, when a p-polarized laser pulse is obliquely incident on a vacuum–plasma interface, SH can be generated in the absence of magnetic field and or any required conditions for phase matching (Jha & Agrawal, Reference Jha and Agrawal2014). Generation of phase-mismatch second and third harmonics has been studied in the interaction of an intense laser pulse with strongly magnetized dense plasma, and it is shown that the harmonic efficiencies can be increased by magnetic field (Ghorbanalilu, Reference Ghorbanalilu2012). In addition, generation of phase-mismatch SH radiation in the reflected component of vacuum–plasma interface by using a s-polarized laser pulse have been reported (Parashar & Sharma, Reference Parashar and Sharma1998; Singh et al., Reference Singh, Gupta, Yadav and Tripathi2005).
The experimental and theoretical investigation approved strong SH generation in Argon gas by focused spatiotemporal femtosecond laser pulses (Li et al., Reference Li, Ni, Xie, Zeng, Yao, Chu, Zhang, Jing, He, Xu, Cheng and Xu2014). On the other hand, second and third-harmonic generations from magnetic metamaterials have been observed under normal and oblique incidences of femtosecond Gaussian laser pulse (Klein et al., Reference Klein, Wegener, Feth and Linden2007). Furthermore, SH radiation from underdense plasma has already been observed in past decades (Mori et al, Reference Mori, Shiraishi, Abe, Taki, Kawada and Kondo2002; Giulietti et al., Reference Giulietti, Banfi, Deha, Giulietti, Lucchesi, Nocera and Zun2009). Moreover, the recent observation approves the SH generation in the laser interaction with plasma–vacuum boundary (Yeung et al. Reference Yeung, Rykovanov, Bierbach, Li, Eckner, Kuschel, Woldegeorgis, Rödel, Sävert, Paulus, Coughlan, Dromey and Zepf2017).
The brief history of SH generation shows that this phenomena has been studied by many authors. They have investigated the SH generation inside the plasma or in the vacuum. In view of this fact that in a real physical system the SH can be generated inside the plasma as well as vacuum due to the laser pulse interaction with plasma surface, we would like to investigate the generation of SH in both sides of the plasma–vacuum boundary simultaneously. The results presented in this paper not only confirm the previous reports, but also can be modified and generalized to a magnetized plasma. On the other hand, results show that the SH power is less than that the previous reports for a non-magnetized plasma if the transmitted and reflected SH radiations are considered simultaneously. We show that deviation with previous reports enhances by increasing the laser intensity and plasma density. The model is valid for underdense plasma $({\rm \omega} _{\rm p}^2 /{\rm \omega} _0^2 \,{\rm \ll}\, 1)$ in the weakly relativistic regime (I 0 ≤ 1017 W/cm2 and or $a_0^2 \,{\rm \ll}\, 1$ ) for angle of incidence varying from 0° up to critical angle. It is lucid that beyond the critical angle, propagation constant becomes imaginary number and the laser propagation becomes evanescent.
The organization of this paper is as follows: In the next section, we derive the equation for non-linear current density as a source of SH generation. The study is undertaken in the mildly relativistic regime, using a perturbative approach. In Section 3, we obtain the amplitudes of transmitted and reflected SH radiations. The SH conversion efficiency, for both transmitted and reflected components, is presented in Section 4, and the influences of incidence angle, magnetic field strength, and plasma density on SH power are investigated. The conclusion is summarized in Section 5.
2. FORMULATION AND GOVERNING EQUATIONS
Consider a vacuum–plasma interface at z = 0; z < 0 being vacuum and z > 0 a uniform underdense plasma of density n 0 that is set in a ${\bf B}( = B_0\hat y)$ transverse magnetic field. A p-polarized laser beam (propagating in the x–z plane) incidents on the interface at an angle of incidence θ as shown in Figure 1.
where E 0 is the amplitude of the incident electric field, k 0x = (ω0/c)sin θ and k 0z = (ω0/c)cos θ are the wavenumber components along the x and z directions, respectively. The electric and magnetic fields of the transmitted laser can be written as
where k 1x = k 0x , $k_{1z} = ({\rm \omega} _0^2 /c^2{\rm \epsilon} _1 - k_{1x}^2 )^{1/2}$ , and ${\rm \epsilon} _1 = k_1^2 c^2/{\rm \omega} _0^2 $ is the dielectric constant at frequency ω0. $E_1 = 2\sqrt {{\rm \epsilon} _1} E_0/({\rm \epsilon} _1+ \sqrt {{\rm \epsilon} _1 - \mathop {\sin} \nolimits^2 {\rm \theta}} /\cos {\rm \theta} )$ is the amplitude of the fundamental electric field transmitted into the plasma. The SH electric field can be written as
where k 2x = (2ω0sin θ)/c, $k_{2z} = (4{\rm \omega} _0^2 /c^2{\rm \epsilon} _2 - k_{2x}^2 )^{1/2}$ . Furthermore ${\rm \epsilon} _2 = k_2^2 c^2/4{\rm \omega} _0^2 $ and E 2 are the dielectric constants at frequency 2ω0 and the SH wave amplitude, respectively. The wave equation governing the propagation of electromagnetic waves through the plasma is given by
where J is the plasma electron current density. The governed equations on electron motion are given by the set of relativistic cold electron fluid equation
and the continuity equation
where γ is the relativistic factor, v and n are the velocity and density of plasma electrons, B and B 0 are the magnetic fields corresponding to the radiation laser pulse and a self-generated magnetic field. We would like to start with perturbative theory and expand all quantities in orders of the radiation field amplitude. By making use of Eq. (6), the velocity components in the x and z directions are, respectively, given by
and
where ωc(= eB 0/mc) represents the cyclotron frequency and E x,z = E 1(x,z) + E 2(x,z) in which E 1(x,z) and E 2(x,z) are the amplitudes of electric field in fundamental and SH. By making use of Eqs (2)–(4), we can solve Eqs (8) and (9) to derive the first order of velocity components as
Where a j(x,z) = eE j(x,z)/mω0 c (j = 1,2) are the components of normalized amplitude of the transmitted fundamental and SH electric field.
By following the same steps, the expression for velocity components in second order is given by
and
The second-order velocity components are obtained by using of Eqs (10) and (11) and simultaneous solutions of Eqs (12) and (13) as bellow
Using Eq. (7), the first-order density perturbation is given as follows
We find from Eq. (16) that the density perturbation disappears in the absence of external magnetic field. The plasma current density ${\bf J} = - en{\bi v}$ components can be derived as
and
Substituting the linear parts of current density into the wave equation, we get to the linear dispersion relations for fundamental and SH.
and
Equations (19) and (20) introduce the dispersion relation for extraordinary waves in fundamental and SH propagating perpendicular to the magnetic field.
3. SH GENERATION
In order to evaluate the amplitude of the SH field, the source currents, Eqs (17) and (18), can be used in the wave Eq. (5) and equate the SH terms on both sides,
and
where
In this case, the wavenumber of the SH is more than twice as large as that for the fundamental wave at which Δk = 2k 1z − k 2z is called the wavevector mismatch for SH radiation. We assume that ∂a 2(x,z)(z)/∂z considerably changes larger than the laser wavelength, means that ∂2 a 2(x,z)(z)/∂z 2 ≪ k 2z ∂a 2(x,z)(z)/∂z, which is known as the slowly varying envelope approximation (SVEA) and is almost valid in non-linear processes. Furthermore, assuming a 1(x,z) depletes very slightly with z so that the quantity $a_{1(x,z)}^2 $ can be considered to be independent of z. Therefore, solution or Eqs (21) and (22) lead us to the normalized amplitudes for the phase-mismatch SH inside the plasma and vacuum as
and
where
Here A 2r and $A_{2{\rm r}}^{\prime} $ are reflected SH amplitudes in x and z directions and a 2x (0) and a 2z (0) refer to the amplitudes of SH wave components at z = 0. Using $\nabla. a_2 = 0$ in the vacuum, we find $A_{2{\rm r}}^{\prime} = (k_{0x}/k_{0z})A_{2{\rm r}}$ . The magnetic field amplitude of the SH radiation derived as
where
In order to obtain the amplitudes a 2x (0), a 2z (0), and A 2r, we apply the proper boundary conditions for electric and magnetic fields E 2x and B 2y and displacement vector εE 2z at z = 0. We get
Integrating the Poisson equation $\nabla. {\rm \epsilon} {\bf E} = - en_1$ , we will get the following relation
The right-hand side of Eq. (28) is very small for underdense plasma $({\rm \omega} _{\rm p}^2 /{\rm \omega} _0^2 {\rm \ll} 1)$ , and we can neglect from this term. Therefore, we obtain from the set of Eqs (26–28) the SH waves amplitudes at plasma surface as
and
The well-known SH conversion efficiency (η) is given by
where ${\rm \mu} _1 = \sqrt {{\rm \epsilon} _1} $ and ${\rm \mu} _2 = \sqrt {{\rm \epsilon} _2} $ are the refractive indexes corresponding to the fundamental and SH radiations, respectively.
3.1 Normal incidence
It is straightforward to show that for normal incidence of laser pulse, the coefficients χ2, χ3, and χ5 do not appear in differential Eqs (21) and (22). Furthermore, just the x component of SH wave and y component of wavevector exist. Therefore, coupled Eqs (21) and (22) reduce to an differential equation for laser field amplitude in x direction as bellow
where the coefficient χ4 is changed to
The detailed derivation of Eq. (32) is shown in Appendix. We obtain the transmitted SH radiation amplitude by solution of Eq. (32) at normal incidence as bellow
Following Eqs (23), (25)–(27), for normal incidence, a 2(0) can be derived as bellow
Above equations show that the amplitude of SH radiation is different from previous report by Jha et al. (Reference Jha, Mishra, Raj and Upadhyay2007). This difference is due to the reflection of SH radiation from vacuum–plasma interface, and changes by plasma density, strength of magnetic field, and laser intensity. Furthermore, the reflected SH radiation amplitude at normal incidence is given by
Therefore, we obtain conversion efficiencies of the SH in both sides of plasma boundary as
It is obvious from Eq. (36), the first term is in complete agreement with Jha et al. (Reference Jha, Mishra, Raj and Upadhyay2007), and the second and third terms are obtained by taking into account the reflected SH components contribution.
3.2 Non-magnetized plasma
It is clear that in the absence of the magnetic field the coefficients of χ2 and χ3 are zero and the other coefficients change to
In this case, the dispersion relations of fundamental and SH waves are expressed by Eqs (19) and (20) with ωc = 0. After applying these changes in Eqs (23–30), the transmitted and reflected SH radiation amplitude are written as
and
where
We get the conversion efficiencies of the SH inside the plasma as well as vacuum as bellow:
It is obvious from Eq. (38), for B = C = 0, the SH efficiency is in complete agreement with Jha and Agrawal (Reference Jha and Agrawal2014).
It should be noted that, Eq. (40) is obtained by taking into account the reflected SH components contribution. Consequently, the introduced SH conversion efficiency by Eq. (40) is different with previous report in which the reflected SH contribution was missed (Jha & Agrawal, Reference Jha and Agrawal2014). The order of deviation will be discussed in the next section.
4. NUMERICAL RESULTS
In this section, we would like to determine the conversion of a fraction of a laser beam to its phase-mismatch SH. To do this, we consider the pump laser a Nd:Yag with intensity I 0 ≤ 1017 W/cm2 (a 0 ≤ 0.3) and frequency ω0 = 1.88 × 1015 rad/s and or wavelength λ = 1 μm.
Figure 2 depicted variation of conversion efficiency $({\rm \eta} \% )$ with respect to the normalized propagation distance z/λ. Figure 2 shows that the conversion efficiency is periodic in z for a given value of Δk, so we have the points with maximum and minimum electric field amplitudes for the SH radiation. The maximum power efficiency (ηmax) takes place in the coherence length z c = π/Δk. In Figure 2a, 2b, the red dashed and black dotted lines are plotted based on the previous report (Jha & Agrawal, Reference Jha and Agrawal2014) and Eq. (40), in the absence of magnetic field, respectively. It seems from the figure that for incidence angle near the critical, the deviation increases; however, for angle far from the critical (Fig. 2a), our result is in complete agreement with previous report.
In Figure 3, we plotted the relative difference of the maximum efficiency ( $\Delta {\rm \eta} _{{\rm max}} = \vert{{\rm \eta} ^{\prime}}_{{\rm max}} - {\rm \eta} _{{\rm max}}\vert /\bar {\rm \eta} _{{\rm max}}$ ), where ${{\rm \eta} ^{\prime}}_{{\rm max}}$ and ηmax refer to the maximum efficiencies reported based on Jha and Agrawal (Reference Jha and Agrawal2014) and Eq. (40) also $\bar {\rm \eta} _{{\rm max}} = ({{\rm \eta} ^{\prime}}_{{\rm max}} + {\rm \eta}_{{\rm max}})/2$ , as a function of incidence angle. We found from the figure that the deviation reaches to the maximum around 10%, near to the critical angle. The results show that deviation depends strongly to the laser field intensity and plasma density, too. For example, for a 0 = 0.3 and plasma density near ωp/ω0 = 0.5, deviation can be increased up to the 36%, which is considerably large.
Figure 4 reveals the influence of self-generated transverse magnetic field on the SH power. The figure indicates SH variation in terms of the normalized propagation distance z/λ. The dashed and solid lines are plotted for a non-magnetized and a magnetized plasma, respectively. It is understood that the maximum conversion efficiency is decreased by magnetic field. Taking into account this fact that such strong magnetic fields can be generated in laser plasma interaction, therefore, we expect that in a real physical system, the SH power becomes less than the power reported for a non-magnetized plasma (Jha & Agrawal, Reference Jha and Agrawal2014).
We compare SH conversion efficiency for normally and obliquely incident of a laser pulse on vacuum–plasma interface in Figure 5, in terms of the self-generated magnetic field strength ωc/ω0. Figure 5a is in complete agreement with previous report (Jha et al., Reference Jha, Mishra, Raj and Upadhyay2007). It seems that the magnetic field intensifies the SH power for normal incidence of a laser pulse, while SH power is weakened by magnetic field for obliquely incident. Moreover, Figure 5 clearly shows that the order of SH power is ten times greater for obliquely incident. Figure 5a demonstrates that the magnetic field is essentially required for SH generation in normal incidence of a laser pulse on plasma surface (Jha et al., Reference Jha, Mishra, Raj and Upadhyay2007).
Figure 6 shows variations of transmitted maximum conversion efficiency $({\rm \eta} _{{\rm max}}\% )$ and reflected conversion efficiency $({\rm \eta} \% )$ in terms of incident angle varying from θ ≈ 0° up to critical angle for different values of ωc/ω0. The solid and dashed lines are plotted for a magnetized and non-magnetized plasmas. Figure 6a shows that the SH power is smaller in a magnetized plasma. As the figures show that the efficiency of SH radiation increases very smoothly with incidence angle, however, it drastically increases near the critical angle. Figure 6b indicates that the influence of magnetic field, on the reflected SH power, is very poor and just near the critical angle a minor decrement ( $ \approx\!\! 1\% $ ) is observable.
In Figure 7, we plotted variations of transmitted maximum conversion efficiency $({\rm \eta} _{{\rm max}}\% )$ and reflected conversion efficiency $({\rm \eta} \% )$ as a function of plasma density ωp/ω0 for different values of incident angle. This figure predicts that for a given angle of incidence θ and magnetic field strength, the SH power sharply increases for both transmitted and reflected components when the plasma density satisfies the required condition θ ≈ θc. For example, for given parameters in Figure 7, the condition θ ≈ θc is satisfied for angles θ = 83° and θ = 77° in plasma densities ωp/ω0 ≈ 0.1 and ωp/ω0 ≈ 0.2, respectively. We find from the Figures 6 and 7, the transmitted SH power is more than twice with respect to the reflected component; however, reflected component is more appropriate for technical and experimental applications.
5. SUMMERY AND CONCLUSION
In conclusion, we investigated the possibility of SH generation in the interaction of an obliquely p-polarized laser pulse on a vacuum-magnetized plasma interface. In view of this fact that strong megagauss magnetic fields can be generated in a laser plasma interaction, we modeled the self-generated magnetic field as a transverse magnetic field. We focused our attention to transmitted as well as reflected SH components. We shown that if the transmitted and reflected SH are considered as a simultaneous process, the results deviated from previous reports, especially near the critical angle (Jha et al., Reference Jha, Mishra, Raj and Upadhyay2007; Jha & Agrawal, Reference Jha and Agrawal2014). The deviation can be increased by laser intensity and plasma density. Our analysis revealed a sharp increase for both transmitted and reflected SH components near the critical angle. We have demonstrated that transverse magnetic field had destructive role and the SH power decreased slightly with magnetic field strength enhancement. The analytical investigations show that the transmitted and reflected SH amplitudes are proportional to laser intensity ( $I \propto a_1^2 $ ), which as expected. If we kept the angel of incident and magnetic field strength constant and changed the plasma density, we found that the SH power for both transmitted and reflected components sharply intensified when the angle of incidence satisfied the required condition θ ≈ θc. In view of this fact that the critical angle reduced by increasing plasma density, for a large incident angle the maximum power is generated at smaller plasma density. A comparison between transmitted and reflected SH revealed that the conversion efficiency is more than twice for transmitted component; however, the reflected component is more proper for technical and experimental applications.
APPENDIX A. Derivation of second harmonic radiation amplitude at normal incidence
A p-polarized laser beam incidents on the interface normally as follow
The electric and magnetic fields of the transmitted laser can be written as
where $E_1 = 2E_0/1 + \sqrt {{\rm \epsilon} _1} $ is the amplitude of the fundamental electric field transmitted into the plasma. The SH electric field can be written as
Using Eq. (6), the first order of velocity components in the x and z directions are, respectively, given by
By following the same steps, the expression for the second-order transverse velocity are given by
By using Eq. (7), the first-order plasma electron density is given as follows
The transverse current density can be derived by using electron density and velocity as follows
By substituting the current density into the wave Eq. (5), we obtain the following expressions
and
In order to determine the amplitude of SH field, Eq. (A.9) can be used in Eq. (5). We arrive
where Δk = 2k 1 − k 2. Using SVEA approximation in above equation, we found