1. INTRODUCTION
Harmonic generation continues to be a fascinating field of research due to its various applications. Second harmonic generation (SHG) (Gupta et al., Reference Gupta, Sharma and Mahmoud2007; Sharma & Sharma, Reference Sharma and Sharma2009; Abdelli et al., Reference Abdelli, Khalfaoui and Ghohrini1992; Liu & Tripathi, Reference Liu and Tripathi1996; Giulietti, et al., Reference Giulietti, Banfi, Deha, Giulietti, Lucchesi, Nocera and Ze Zun1988; Upadhyay & Tripathi, Reference Upadhyay and Tripahi2005; Hafeez et al., Reference Hafeez, Shaikh and Baig2008; Ozaki et al., Reference Ozaki, Bom, Ganeev, Kieffer, Suzuki and Kuroda2007, Reference Ozaki, Bom and Ganeev2008; Liu et al., Reference Liu, Umstadter, Esarey and Ting1993; Huillier & Balcou, Reference Huillier and Balcou1993) has become one of the most investigated and discussed nonlinear optical process since 1961, when Franken et al. (Reference Franken, Hill, Peters and Weinreich1961) experimentally discovered SHG. The primary reason to investigate SHG has consistently been the achievement of efficient frequency doubling, the emphasis has been on phase-matched interaction between the fundamental and second harmonic beam. Phase matching is a condition that essentially requires conversion of linear momentum that also facilitates energy flow from the pump to the second harmonic signal. Experiments on electron and ion acceleration in a laser pulse field using sources of super intense radiation require high time contrast of femtosecond pulses. An efficient way to enhance the contrast is a nonlinear optical process of SHG. Second harmonic generation signals have well-defined polarizations, and thus SHG polarization anisotropy can be used to determine the orientation of proteins in tissues. It can be used in studying buried interfaces, as most surface science techniques cannot access such structures. SHG can provide information of the electric field at an interface. It allows the penetration of the laser power into the overdense region and provides a valuable diagnostics (Merdji et al., Reference Merdji, Guizard, Martin, Petite, Que're', Carre', Hergott, De' roff, Salie'res, Gobert, Meynadier and Perdrix2000; Verma et al., 2009; Panwar et al., 2009; Prasad et al., 2009) of various plasma processes (Dromey et al., Reference Dromey, Bellei, Carroll, Clarke, Green, Kar, Kneip, Markey, Nagel, Willingale, McKenna, Neely, Najmudin, Krushelnick, Norreys and Zepf2009; Hafeez et al., Reference Hafeez, Shaikh and Baig2008). It also provides information about linear mode conversion of the laser into a plasma wave near the critical layer. It has been observed that the uniform plasmas cannot produce even harmonics neither by a plane nor by a circularly polarized electromagnetic wave. In most laser interactions with homogeneous plasma, odd harmonics are generated (Mori et al., Reference Mori, Decker and Leemans1993; Zeng et al., Reference Zens, Shen, Yu and Xu1996). Even harmonics can be produced in the presence of density gradient at an angle to the direction of the wave propagation (Esaray et al., Reference Esarey, Ting, Sprangle, Umstadter and Liu1993; Malka et al., Reference Malka, Modena, Najmudin, Dangor, Clayton, Marsh, Joshi, Danson, Neely and Walsh1997).
The current investigations are dealing with the study of pulsed SHG under condition of phase and group velocity mismatch, and low conversion efficiencies and pump intensities, in negative index materials called artificially engineered meta-materials (Ramakrishna, Reference Ramakrishna2005; Wang et al., Reference Wang, Luo, Peng, Huangfu, Jiang, Wang, Chen and Ran2009). Ultraviolet and X-ray SHG (Chen et al., Reference Chen, Zitter and Tao1995) in semiconductors have been reported, which shows that the subject is of interest for the purpose of realizing coherent sources. Centini et al. (Reference Centini, Roppo, Fazio, Pettazzi, Sibilia, Haus, Foreman, Akozbek, Bloemer and Scalora2008) shown theoretically and experimentally the inhibition of linear absorption for phase and group velocity mismatch second and third harmonic generation in strongly absorbing materials, GaAs, in particular, at frequency above the absorption edge. Schifano et al. (Reference Schifano, Baton, Biancalana, Giuletti, Giuletti, Labaune and Renard1994) experimentally investigated the properties of the second harmonic emission and tested the effectiveness of this emission as a diagnostics for plasma inhomogenities induced by filamentation. Mironov et al. (Reference Mironov, Lozhkarev, Ginzburg and Khazanov2009) recently observed the effect of instantaneous cubic nonlinearity on SHG of femtosecond laser pulses. They have also analyzed the possibility of improving generation efficiency and shortening pulse duration. He observed 60% energy conversion efficiency and showed that the additional correction of spectral phase at the SH significantly reduces pulse duration. Shen (Reference Shen1989) has shown that SHG is a versatile tool for studies of many kinds of surfaces and interfaces. Ultrashort laser pulses can be used to monitor surface dynamics and reaction with sub-picoseconds time resolution. Krushelnik et al. (Reference Krushelnick, Ting, Burris, Fisher, Manka and Esarey1995) observed second harmonic shifted by the plasma frequency giving information about the stimulated Raman process. Liu et al. (Reference Liu, Umstadter, Esarey and Ting1993) have observed harmonic generation using a 1 ps, 1 µm, variable intensity laser in hydrogen gas jet plasma produced by tunnel ionization. Parashar & Sharma (Reference Parashar and Sharma1998) have studied SHG by an obliquely incident laser on a vacuum-plasma interface and rippled metal surface. Dahiya et al. (Reference Dahiya, Sajal and Sharma2007) presented particle-in-cell (PIC) simulations of phase matched second and third harmonic in ripple density plasmas. Yadav et al. (2008) have investigated stimulated Compton scattering (SCS) and stimulated Brillion scattering (SBS) of second harmonic signals. Salih et al. (2003) have studied SHG in self-created magnetized plasmas. The harmonic amplitude shows resonant enhancement as ωc tends to ω. Kaur and Sharma (Reference Kaur and Sharma2009) and Kura et al. (Reference Kaur, Sharma and Salih2009) have shown in a collisional magnetoplasma the self-defocusing of the laser causes reduction in the efficiency of second harmonic generation. Recently Verma and Sharma (Reference Verma and Sharma2009) developed a paraxial theory of third harmonic generation by a finite spot size laser in a tunnel ionizing gas.
In this paper, we study the generation of second harmonic in the presence of magnetic field. Physical mechanism of generation of second harmonic is as follows: laser propagating through the plasma imparts oscillatory velocity on electrons and exerts a pondromotive force on them. This pondromotive force produces nonlinear oscillatory velocity at 2ω and then produces nonlinear current at 2ω frequency, hence second harmonic current is produced. In Section 2, we have calculated the linear and nonlinear current densities, and in Section 3 amplitude of second harmonic generation is calculated. Finally, in Section 4, we discuss the results.
2. CALCULATION OF LINEAR AND NONLINEAR CURRENT DENSITIES
Consider a laser produced plasma with rippled density n 0 = n 00 + n q, n q = n 0qe iqz, and sheared magnetic field,
The magnetic field resembles azimuthal magnetic field in the slab model. A laser propagates through the plasma with electric field
It imparts oscillatory velocity to electrons,
where -e is the electronic charge, m is the mass of electron, and ω is the frequency of the laser, and we have assumed ω≫eB 0/m. The laser also exerts a second harmonic ponderomotive force on electrons
where
The electron response to is governed by
Replacing ∇ by ik and by −iω, we get
The nonlinear second harmonic current density at (2ω, 2k+q) can be written as
One may note that the transverse component of second harmonic current density, J 2ω xNL, scales as ωc, i.e., it is proportional to x, hence is zero on laser axis.
The linear response of electrons to the self-consistent second harmonic field is governed by
Taking
one obtains
where we have assumed The linear current density at 2ω can be written as
3. SECOND HARMONIC GENERATION
The wave equation governing is
where
Since has fast variation along and slow in , i.e. , we get from the z component of Eq. (10)
Using this value in the x component of Eq. (10) we get
Using the values of from above we may write
where , and . Then Eq. (12) can be written as
where
Writing
where k 2 = 2k + q, Eq. (14) can be written as
The phase matching condition for resonant second harmonic generation is
If right-hand-side of Eq. (17) is ignored, it resembles the Harmonic oscillator equation,
with and The above equation has bounded solutions. The first two Eigen modes with corresponding eigen values are
Since R 0 is proportional to x, the coupling of only n = 1 mode of the second harmonic to the pump is relevant. In the presence of right-hand-side in Eq. (17), we presume that the mode structure of E 2ω remains the same but amplitude acquires a z-dependence. Thus, we write
where
substituting this in Eq. (17) multiplying the resulting equation by Fdx and integrating over x from −∞ to ∞, we get
where
After solving it we get
The normalized second harmonic amplitude can be written as
where
with and A 0 = amplitude of the laser.
We have solved Eq. (24) numerically for the following parameters: ωc0/ω = 0.2, 0.4, a 0 = 0.4, n q0/n 00 = 0.3, ωp2/ω2 = 0.05, 0.1 and ωpz/c = 1000.
In Figure 1, we have plotted the normalized second harmonic amplitude as a function ωpr 0/c for ωc0/ω = 0.2, and 0.4. At small laser spot size, the ratio of second harmonic amplitude to the amplitude of the fundamental wave is low as the electromagnetic modes are strongly localized. As the laser spot size grows, the no local effects. As the laser spot size grows, the nonlocal effects become important and magnetic field effects are there. As magnetic field increases i.e., ωc0/ω from 0.2 to 0.4 second harmonic generations become fast and its normalized amplitude increases from 0.09 to 0.185. This is due to the fact that as the laser goes into the plasma its spot size increases and magnetic field coupling becomes stronger and hence nonlinearity increases. Thus, more and more second harmonic generates. After some value of ωp r 0/c generation of second harmonic saturates. Since as the spot size becomes larger, non-local effects become un- important and hence the amplitude of the second harmonic saturates. In Figure 2, variation in normalized second harmonic amplitude is plotted with ωp r 0/c for different values of ωp2/ω2 = 0.05 and 0.1. Figure 2 shows that as the electron density increases more and more, the second harmonic generates likewise. By increasing the electron density, the nonlinearity increases. As SHG is a nonlinear phenomenon, it increases more and more. As ωp2/ω2 increases from = 0.05 to = 0.1 the amplitude of second harmonic increases from 0.135 to 0.195.
4. DISCUSSION
Second harmonic signals are very useful in reading DVD's as they can read a four times smaller area than the fundamental signal of the laser. We find that as magnetic field increases, generation of second harmonic becomes faster. This happens due to the strong coupling between magnetic field and laser field. Here ripple density provides phase matching between fundamental and second harmonic beam. Phase matching is a condition that essentially requires conversion of linear momentum that also facilitates energy flow from the pump to the second harmonic signal. Hence, more and more second harmonic generates. Electron density also plays important role since as electron density increases for particular value of magnetic field nonlinearity increases and hence second harmonic generation increases.
ACKNOWLEDGEMENT
The authors are grateful to Prof. V.K. Tripathi, IIT Delhi for fruitful discussions. The author is very thankful to the CSIR for financial support.